4.1 This test method can be extended to use any material that has the necessary nuclear and activation properties that suit the experimenter's particular situation. No attempt has been made to fully describe the myriad problems of counting techniques, neutron-fluence depression, and thick-foil self-shielding. It is assumed that the experimenter will refer to existing literature on these subjects. This test method does offer a referee technique (the standard gold foil) to aid the experimenter when they are in doubt of their ability to perform the radiometric technique with sufficient accuracy.

4.2 The standard comparison technique uses a set of foils that are as nearly identical as possible in shape and mass. The foils are fabricated from any material that activates by an (n, γ) reaction, preferably having a cross section approximately inversely proportional to neutron speed in the thermal energy range. Some of the foils are irradiated in a known neutron field (at NIST) or other standards laboratory). The foils are counted in a fixed geometry on a stable radiation-detecting instrument. The neutron-induced reaction rate of the foils is computed from the counting data, and the ratio of the known neutron fluence rate to the computed reaction rate is determined. For any given foil, neutron energy spectrum, and counting set-up, this ratio is a constant. Other foils from the identical set can now be exposed to an unknown neutron field. The magnitude of the fluence rate in the unknown field can be obtained by comparing the reaction rates as determined from the counting data from the unknown and reference field, with proper corrections to account for spectral differences between the two fields (see Section 5). One important feature of this technique is that it eliminates the need for knowing the detector efficiency.

4.3 This test method follows the Stoughton and Halperin convention for reporting thermal neutron fluence. Other conventions are the Wescott convention (followed in Test Method E481) and the Hogdahl convention. Practice E261 explains the three conventions and gives conversion formulae relating values determined by the different conventions. Reference (1)3 discusses the three thermal-neutron conventions in detail.

1.1 The purpose of this test method is to define a general procedure for determining an unknown thermal-neutron fluence rate by neutron activation techniques. It is not practicable to describe completely a technique applicable to the large number of experimental situations that require the measurement of a thermal-neutron fluence rate. Therefore, this method is presented so that the user may adapt to their particular situation the fundamental procedures of the following techniques.

1.1.1 Radiometric counting technique using pure cobalt, pure gold, pure indium, cobalt-aluminum, alloy, gold-aluminum alloy, or indium-aluminum alloy.

1.1.2 Standard comparison technique using pure gold, or gold-aluminum alloy, and

1.1.3 Secondary standard comparison techniques using pure indium, indium-aluminum alloy, pure dysprosium, or dysprosium-aluminum alloy.

1.2 The techniques presented are limited to measurements at room temperatures. However, special problems when making thermal-neutron fluence rate measurements in high-temperature environments are discussed in 9.2. For those circumstances where the use of cadmium as a thermal shield is undesirable because of potential spectrum perturbations or of temperatures above the melting point of cadmium, the method described in Test Method E481 can be used in some cases. Alternatively, gadolinium filters may be used instead of cadmium. For high temperature applications in which aluminum alloys are unsuitable, other alloys such as cobalt-nickel or cobalt-vanadium have been used.

1.3 This test method may be used to determine the equivalent 2200 m/s fluence rate. The accurate determination of the actual thermal neutron fluence rate requires knowledge of the neutron temperature, and determination of the neutron temperature is not within the scope of the standard.

1.4 The techniques presented are suitable only for neutron fields having a significant thermal neutron component, in which moderating materials are present, and for which the average scattering cross section is large compared to the average absorption cross section in the thermal neutron energy range.

1.5 Table 1 indicates the useful neutron-fluence ranges for each detector material.

TABLE 1 Useful Neutron Fluence Ranges of Foil Material

Foil Material

Form

≈ Useful Range (neutrons/cm ²)

Indium

pure or alloyed with aluminum

10³ to 10¹²

Gold

pure or alloyed with aluminum

10⁷ to 10¹⁴

Dysprosium

pure or alloyed with aluminum

10³ to 10¹⁰

Cobalt

pure or alloyed with aluminum

10¹⁴ to 10²⁰

1.6 This standard does not purport to address all of the safety concerns, if any, associated with its use. It is the responsibility of the user of this standard to establish appropriate safety, health and environmental practices and determine the applicability of regulatory limitations prior to use.

1.7 This international standard was developed in accordance with internationally recognized principles on standardization established in the Decision on Principles for the Development of International Standards, Guides and Recommendations issued by the World Trade Organization Technical Barriers to Trade (TBT) Committee.